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Surface Plasmon Enhanced Nitrogen-Doped Graphene Quantum Dot Emission by Single Bismuth Telluride Nanoplates

Saleem U.a,b, Permatasari F.A.c,d, Iskandar F.d, Ogi T.c, Okuyama K.c, Darma Y.d, Zhao M.e, Loh K.P.e, Rusydi A.e, Coquet P.a, Birowosuto M.D.a,f, Wang H.a,b

a CINTRA – CNRS/NTU/Thales, UMI 3288, 637553, Singapore
b School of Electrical and Electronics Engineering, Nanyang Technological University, 639798, Singapore
c Department of Chemical Engineering, Graduate School of Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan
d Department of Physics, Faculty of Mathematics and Natural Sciences, Institut Teknologi Bandung, Bandung, 40132, Indonesia
e Department of Chemistry, National University of Singapore, 117543, Singapore
f Physics Research Center, The Indonesian Institute of Sciences, Puspitek, Serpong, 15314, Indonesia

[vc_row][vc_column][vc_row_inner][vc_column_inner][vc_separator css=”.vc_custom_1624529070653{padding-top: 30px !important;padding-bottom: 30px !important;}”][/vc_column_inner][/vc_row_inner][vc_row_inner layout=”boxed”][vc_column_inner width=”3/4″ css=”.vc_custom_1624695412187{border-right-width: 1px !important;border-right-color: #dddddd !important;border-right-style: solid !important;border-radius: 1px !important;}”][vc_empty_space][megatron_heading title=”Abstract” size=”size-sm” text_align=”text-left”][vc_column_text]© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, WeinheimThe light–matter interaction between nitrogen-doped graphene quantum dots (N-GQDs) and bismuth telluride (Bi2Te3) nanoplates is investigated. A maximum of (2.9 ± 0.3)-fold emission rate enhancement is observed at room temperature due to the coupling of N-GQD emission with the breathing mode of surface plasmon of single Bi2Te3 nanoplates. The enhancement varies with different emission wavelengths and nanoplate diameters in accordance with results obtained through the dipole radiation power in the electromagnetic simulations. From experiment, the quantum yield of N-GQDs is obtained to be almost unity, while Bi2Te3 nanoplates may replace the conventional antenna. Such combination of novel active and plasmonic materials is promising for efficient lighting applications with multiple functionalities, especially tunable plasmonic metamaterial based on topological insulators.[/vc_column_text][vc_empty_space][vc_separator css=”.vc_custom_1624528584150{padding-top: 25px !important;padding-bottom: 25px !important;}”][vc_empty_space][megatron_heading title=”Author keywords” size=”size-sm” text_align=”text-left”][vc_column_text]Bismuth telluride,Electromagnetic simulation,Light-matter interactions,Nanoplates,Nitrogen doped graphene,Plasmonic metamaterials,Surface plasmons,Topological insulators[/vc_column_text][vc_empty_space][vc_separator css=”.vc_custom_1624528584150{padding-top: 25px !important;padding-bottom: 25px !important;}”][vc_empty_space][megatron_heading title=”Indexed keywords” size=”size-sm” text_align=”text-left”][vc_column_text]bismuth telluride,emission,graphene quantum dots,nanoplates,surface plasmons[/vc_column_text][vc_empty_space][vc_separator css=”.vc_custom_1624528584150{padding-top: 25px !important;padding-bottom: 25px !important;}”][vc_empty_space][megatron_heading title=”Funding details” size=”size-sm” text_align=”text-left”][vc_column_text]The authors acknowledge L. Y. Tobing for his help with the reflection measurements. The authors also acknowledge financial supports from the Ministry of Education (MOE2016-T2-1-052) and the National Research Foundation of Singapore (NRF-CRP12-2013-04), the Japan Society for the Promotion of Science, and the Kemenristek Dikti of Indonesia. Other funding details can be found in the Supporting Information.[/vc_column_text][vc_empty_space][vc_separator css=”.vc_custom_1624528584150{padding-top: 25px !important;padding-bottom: 25px !important;}”][vc_empty_space][megatron_heading title=”DOI” size=”size-sm” text_align=”text-left”][vc_column_text]https://doi.org/10.1002/adom.201700176[/vc_column_text][/vc_column_inner][vc_column_inner width=”1/4″][vc_column_text]Widget Plumx[/vc_column_text][/vc_column_inner][/vc_row_inner][/vc_column][/vc_row][vc_row][vc_column][vc_separator css=”.vc_custom_1624528584150{padding-top: 25px !important;padding-bottom: 25px !important;}”][/vc_column][/vc_row]